To kick off our series of Home Rad Lab articles, it was decided to first delineate the legal parameters of owning and using radioactive sources.
Unfortunately since 9/11 the issue of what is legal and what is not legal
has been in flux, as the US Federal government, especially the Nuclear
Regulatory Commission, has been tightening up the rules and regulations
concerning radioactive materials in general. Many of the regulations issued by
the NRC stem from the Atomic energy Act of 1954, Energy Reorganization Act of 1974, and Uranium Mill Tailings
Radiation Control Act of 1978.
In 2005, the Energy Policy Act of 2005
was passed. Prior to this law, the
NRC had jurisdiction over certain types of radioactive material, and States over
other types. Surprisingly, the NRC had no jurisdiction over Radium! Up until
2005, Radium was regulated only by the individual STATES. This to say the least
was confusing to the layperson, lab operator, and even NRC employees. Not that
an amateur scientist can truly understand all the laws and regulations totally,
we will endeavor to create a safe and sane legal outline that will assure the
instructor or hobbyist at least a basic understanding of the allowable
procedures and experiments.
While the
Energy Policy Act of 2005 was AUTHORITY, until RULES were instituted, the
LAW had nothing to enforce.
http://www.nrc.gov/reading-rm/doc-collections/news/2007/07-052.html
Finally in
April 2007 a definitive set of new rules has emerged, from which we may now
derive guidelines for safe and currently legal radioactive experiments.
Of particular
concern was the eminent reclassification and strict regulation of the most
common radioactive source, the common radium painted watch
hand.
Serious consideration was given to restricting the ownership of radium watch hands to only 50 units at any one location. This of course would have reduced the ability of any institution to own a reasonable amount of that valuable material. Fortunately after long and contentious debate, much input from the public and industrial entities, it has been decided to delete the quantity restrictions on radium watch hands altogether. Currently
NRC regulations prohibit manufacturing any article, device or apparatus from Radium (Ra-226), and the use of preexisting material has its restrictions as well, but basically a vial of Radium watch hands is still OK to own at this time, subject to the general license provided in 10CFR-31.12.
NRC
rules are very different for
A) Individuals
B) Educational
institutions
C) Business entities.
Before we
get into the particulars we must understand some of the basic terminology used
in the radiation lab.
PERSONS -Means (1) any individual, corporation, partnership, firm, association, trust, estate, public or private institution, group or Government agency. 10CFR-40.4
ISOTOPE – Normal atoms have the same
number of Neutrons and Protons in their nucleus. Isotopes include all variations
of the same chemical element that have the same number of Protons, but different
numbers of Neutrons in the nucleus. All isotopes of a particular element have
nearly identical chemical properties, but can have very different radioactive
qualities. All variations of the same element are isotopes, but not all are
radioactive. There are a vast number of radioactive isotopes, many of common
elements like carbon, gold, silver or sodium. Once an atom increases or
decreases the number of Protons in the nucleus, it is no longer the same
element, but has transmuted into a different element altogether. That new
element may have several isotopes all of its own. This fact of nuclear
transmutation is evidenced by careful study of the nuclear decay chains in the
link provided. Uranium-238 literally turns into Thorium which turns into
Protactinium which turns into a different isotope of Uranium, and so on until
stable Lead is the only thing left.
http://www.ead.anl.gov/pub/doc/natural-decay-series.pdf
SOURCE MATERIAL -“SOURCE” in this case means “natural source”. There are three decay chains that exist in nature. These are headed by Uranium-238, Uranium-235 and Thorium-232. Decay chain starts with the parent material and over time, decays into other radioactive material, until after a great deal of time, the final residue is stable lead (Pb). The exact type of stable lead depends on the originating parent material. Radium and Radon are some of the intermediate daughters or PROGENY of these decay chains. Uranium as found in nature, that is un enriched in U-235 is source material, and Depleted Uranium, uranium which has had a portion of the U-235 removed comes under the “source” definition. Any kind of ENRICHED URANIUM- that is uranium with more than .7% U-235 is no longer considered “source”, but is “special nuclear material”- which is forbidden to own by individuals.
10cfr-40.4 Source Material means: (1) Uranium or thorium, or any combination thereof, in any physical or chemical form or (2) ores which contain by weight one-twentieth of one percent (0.05%) or more of: (i) Uranium, (ii) thorium or (iii) any combination thereof. Source material does not include special nuclear material.
Under the new
NRC rules, Radium is now included in this category,
http://www.ead.anl.gov/pub/doc/natural-decay-series.pdf
http://www.nrc.gov/materials/srcmaterial.html
BYPRODUCT MATERIAL- radioactive
material NOT FROM NATURE. Man-Made in an accelerator or reactor.
Under the new
NRC rules, Radium and Uranium plant tailing piles are now included in this
category.
http://www.nrc.gov/reading-rm/doc-collections/fact-sheets/byproduct-materials.html
BYPRODUCT MATERIAL Exempt Sources: Those man made (Byproduct) radioactive materials that are exempt from
licensing in certain quantities, usually supplied to the Home Lab by companies
such as Spectrum Techniques in safe SEALED
SOURCES.
http://www.spectrumtechniques.com/
No man made materials that is not on this list are allowed to be owned
except under license. This includes Plutonium, Americium, and Californium,
basically any element heavier than Uranium on the Periodic Chart of
Elements.
Check out the
full list of approved materials and the allowable quantities under Schedule B
at:
http://www.nrc.gov/reading-rm/doc-collections/cfr/part030/full-text.html
ALL materials
supplied by Spectrum Techniques are of exempt quantity, therefore no
license or special handling is needed.
NRC- US Nuclear Regulatory Commission, the primary regulator of radioactive
materials in the USA.
Click here for
the NRC’s Public Reading Room:
http://www.nrc.gov/reading-rm.html
NRC
AGREEMENT STATES- Those states
that have elected to take primary authority of radiation matters under their own
control. State rules must be at least as restrictive as the NRC’s version. There
are currently 34 Agreement States with others in consideration. Click here to
review your state’s current status:
Non
AGREEMENT STATES - States which
prefer the NRC to be the primary authority in radiation matters. Even these
states have certain responsibilities that they must enforce. Click here to review your state’s
current status:
Misuse- The use of
any radioactive material for other than it’s intended or licensed purpose.
Removing a radioactive Am-241 from a smoke detector for use as a test source is
considered a grievous misuse. Penalties are far beyond any
benefit.
General License- A type
of license automatically granted to and end user to own and operate some devices
containing radioactive materials. The license is granted for the intended use of
these devices only, and does not convey permission to use the device in an
unintended manner (see Misuse). Transfer of such devices is generally forbidden
between unlicensed persons, as is any alteration, removal of radioactive
material or manufacture for sale. A generally licensed device usually consists
of radioactive material contained in a sealed source within a shielded
device
“The general licenses provided in this part are effective without the filing of applications with the Commission or the issuance of licensing documents to particular persons. Specific licenses are issued to named persons upon applications filed pursuant to the regulations in this part”:
http://www.nrc.gov/reading-rm/doc-collections/cfr/part040/part040-0020.html
Perfect examples are: Smoke Detectors (Am-241), Tritium Lights (H3) and
Signs, Static Brushes (Po-210). Depending upon the isotope involved, the only
avenue of transferring the device is through disposal in a landfill. Some
devices must be returned to the manufacturer for proper disposal. Again, an individual cannot sell, resell
or transfer Generally Licensed material without a Specific License to do so.
http://www.nrc.gov/materials/miau/general-use.html#7
Specific License- The type of licensed required to manufacture, process and distribute regulated radioactive material. A University Lab would require a Specific License to own and use certain types or quantities of radioactive materials. This type license is not within the reach of the Home or small School Lab. “Specific licenses are issued to named persons upon applications filed pursuant to the regulations in this part”:
http://www.nrc.gov/reading-rm/doc-collections/cfr/part040/part040-0020.html
We will deal
with only Unlicensed\, Generally Licensed, or Exempt sources.
PART 2-
Radioactive Lab Sources.
As
stewards of the SAFETY of our students, more importantly, the PERCEIVED SAFETY,
we must first and foremost be adamant about using only materials that are
PERFECTLY SAFE UNDER EVERY CIRCUMSTANCE. All the sealed
sources from Spectrum Techniques meet this criteria and I will suggest a few
more that should be suitable. Any items such as Uranium Ore and Gas lantern
Mantles that can leave debris behind should not be taken into a classroom. These
materials are perfectly safe in the Home Lab with only a modicum of caution and
common sense.
Radiation dose to humans is a subject best address by health
professionals, but certain guidelines have been set by the NRC and can be found
here:
http://www.nrc.
Sealed Sources Suitable for classroom- unrestricted. >HIGHLY recommended classroom source<
Listed in order of priority:
|
These first
three |
are basic and are the
|
first three any lab
should |
obtain. |
|
|
Cs137S5 |
5uCi. |
30.1 years |
Gamma, Beta |
32, 661.6, β511.6, β1173.2 |
|
Sr-90S |
0.1uCi. |
28.8 years |
Beta |
β546 |
|
Po-210S |
0.1uCi. |
138 days |
Alpha |
5407.5 |
|
|
|
|
|
|
|
|
|
|
|
|
|
These Isotopes
|
are very useful
|
in slightly advanced |
to advanced experiments |
|
|
Co-60S1 |
1uCi. |
5.27 years |
Gamma, Beta |
1173.2, 1332.5, β317.9 |
|
Tl-204S1 |
1uCi. |
3.78 years |
Beta |
β763.7 |
|
Na-22S1 |
1uCi. |
2.6 years |
Gamma |
1274.5, 511 |
|
Ba-133S1 |
1uCi. |
10.7 years |
Gamma |
81.0, 276.3, 303.7, 355.9, 383.7 |
|
Fe-55S100 |
100uCi. |
2.73 years |
X-ray, Beta |
5.9, 6.5, β231.4 |
|
Cd-109S1 |
1uCi. |
453 days |
Gamma |
88.0 |
|
Eu-152S1 |
1uCi. |
13.5 Years |
Gamma, Beta |
Multiple energies |
|
Cs/ZnS |
1uCi. |
Mixed |
"Unknown" |
32, 661.6, 1115.5 |
|
Co-57S1 |
1uCi. |
270 days |
Gamma |
122.1, 136.4 |
|
Mn-54S1 |
1uCi. |
312 days |
Gamma, Beta |
834.8, β542.2 |
|
C-14S10 |
10uCi. |
5730 years |
Beta |
β156.5 |
|
Zn-65S1 |
1uCi. |
244 days |
Gamma, Beta |
1115.6, β236.34 β1351.9 |
Sealed sources may be purchsed, owned, used and discarded without a license. It takes a license to transfer sealed sources, so you cannot resell or even give them away.
Uranium
Ore > OK in clasrooms if
contained <
Any number of experiments will be discussed using this basic radioactive material. At this time simply owning ore in any quantity is no problem.
Business or educational entities can own and process any amount of uranium ore, yielding up to 15 pounds in one session and 150 pounds in any one year of Yellowcake or concentrated uranium. Per Mr. Charles Cain, Senior Materials Analyst, NRC office, Arlington TX, the office in charge of uranium milling. The US NRC does not regulate mining of uranium ore.
Ownership:
Individuals OK
Any number
of experiments will be discussed using this basic radioactive material. At this
time simply owning ore in any quantity is no problem.
Ownership:
Individuals OK
10CFR-40.13D “b) Any person is exempt from the regulations in this
part and from the requirements for a license set forth in section 62 of the act
to the extent that such person receives, possesses, uses, or transfers unrefined
and unprocessed ore containing source material; provided, that, except as
authorized in a specific license, such person shall not refine or process such
ore.” “(a) A general license is hereby issued authorizing commercial
and industrial firms, research, educational and medical institutions and
Federal, State and local government agencies to use and transfer not more than
fifteen (15) pounds of source material at any one time for research,
development, educational, commercial or operational purposes. A person
authorized to use or transfer source material, pursuant to this general license,
may not receive more than a total of 150 pounds of source material in any one
calendar year.” Mr. Charles Cain,
Senior Materials Analyst at the NRC office in charge of uranium milling and
processing indicates that the NRC does not regulate the mining operation of
uranium ore, and defines the words "source material" in section 40.22 as the end
result of processing, in other words yellowcake. In a telephone
conversation of 26 Ap 2007, he answered some direct questions for
me: Q: How much ore
may a person own? A: Any amount. As much as your dump truck will hold, then go
back for some more. Q: May an individual
who is part of an educational or commercial entity process i.e. concentrate
uranium ore.? A: Yes, up to 15 pounds of yellow cake per session, 150
pounds per year. Educational OK
Business OK
Processing ore to yellowcake i.e.
concentrating:
§ 40.22 Small quantities of
source material.
Ownership:
Individuals OK
Depleted Uranium Metal (DU) >
NOT suitable for classroom. An excellent radioactive material for numerous
experiments in the HOME LAB environment< DU is any uranium with less than
.711% by weight of U-235. DU metal is usually about .2% U-235, the rest is low
radioactivity U-238.
Ownership:
Depending on the item see: http://www.nrc.
Individuals
No
Educational OK
up to 15 pounds
Business OK up
to 15 pounds
Subject to
rules under 10CFR-40.25 see:
http://www.nrc.
Radium/
Ra-226> NOT suitable for classroom. <An excellent
radioactive material for numerous experiments in the HOME LAB environment,
radium watch hands may be used, but only with care. Handling any Radium painted
object WILL transfer Ra-226 to the skin and surroundings. In the school lab, an
intact watch, clock or compass is the ONLY approved source. All glass covering
must be undamaged and full shield the items inside. Never let a student handle
the item. Only qualified instructors should be allowed to handle the item.
Cleanup after a dropped/broken clock could be a financial burden. Far better to
use one of the proven safe test discs from Spectrum Techniques in the classroom
environment. Let me suggest videotaping actual experiments using any radium
painted device. Redefined in 2007 as a BYPRODUCT
MATERIAL.
LINK MR
WIZARD
http://www.mrwizard
“Everyday
Radioactivity” episode.
Ownership:
Exempted see- http://www.nrc.
Educational
OK
Thorium/
Th-232 >OK in classroom if sealed in a container. <
Thorium has
been used in many consumer products in the past. It is still used in an
abundance of everyday items, as it has certain unique characteristics that make
it invaluable. All isotopes of Thorium are radioactive, the most common one
being Th-232, found in many kinds of rocks.
Th-232 is the
head of one of the three natural decay chains, while Thorium-230, 231, 234, and
228 are progeny of decay chains.
Some of the many uses include:
alloying metals for extra strength, used to provide a better filament in high
power radio transmitting tubes, added to welding rods, and making high
temperature ceramics. The most ubiquitous use in the recent past has been in the
form of Thorium Dioxide, ThO2 in the making of Welsbach Gas lantern
mantles.
http://en.wikipedia
Although
the use of Thorium in Gas Mantles has been superseded by Cerium Oxide, many
previously manufactured mantles are still around and may be purchased at a
nominal fee.
Ownership:
Exempted see- http://www.nrc.
Educational OK
Radioactive Potassium-40 /K-40 > Suitable for classrooms-unrestricted. Highly recommended>
Sounds
intimidating, but it is in virtually all soil, most rocks, and fertilizer,
cleaning products, even your own bones. K-40 is not only everywhere; we eat it
in the form of salt-substitute. The food product is actually a useful Home Rad
Lab source! Other foods such as bananas and nuts have a fairly high
concentration too.
Ownership:
unrestricted in the natural state
Individuals
OK
Educational
OK
Business
OK
Uranium
Glass
> Suitable for classroom - unrestricted.
HIGHLY recommended classroom
source.<
“Depression
glass”, uranium glass marbles, other green colored glass items. Perfectly safe,
use a small amount of uranium in the manufacturing process. Also glows under UV
light.
Ownership:
Exempted under http://www.nrc.
Individuals
OK
Educational
OK
Business
OK
FiestaWare, Bauer ceramic dishware, many other ceramics coated with the “radioactive red” glaze> Suitable for classroom - unrestricted. HIGHLY recommended classroom source.<
Ownership:
Exempted under: http://www.nrc.
Individuals
OK
Educational
OK
Business
OK
Future articles
will highlight some of the many everyday items that happen to be radioactive,
such as ceramic dishware, uranium glass dishes and objects, granite countertops,
building materials, soil and many more.
Besides Uranium
(Ore or Autunite in Acrylic), Radium and Thorium samples, I highly recommend the
Home Rad Lab be equipped with at least a Cesium-137 disc (Gamma and Beta
radiation), Strontium-90 disc (Beta only), and a Polonium Disc (Alpha
only).
http://www.spectrum
Most school
science supply houses carry the Spectrum Techniques products.
As our series of experiments evolve and get more complex, other test discs will be used, such as Cobalt-60, Sodium-22, Cadmium-109 and Barium-133. The culmination of the series involves “milking” one radioactive product from another, Ba-137m from Cs-137 using a Spectrum Techniques “Isotope Generator”.
Recap of important points:
Do not remove radioactive material from smoke
detectors.
Do not use any radioactive material in a way inconsistent with the intent
of the object.
PART 3-Home Rad lab Instrumentation
During the course of this series of articles, will be using nuclear instrumentation from the simplest home made apparatus to very sophisticated analytical equipment. I promise that there will be something of interest for everyone.
PART 4-
Human Rad Dose
Radiation dose
to humans is a subject best address by health professionals, but certain
guidelines have been set by the NRC and can be found
here:
http://www.nrc.
No materials used in the Home Rad lab have enough radioactivity to be of any concern.
Have
Fun
George Dowell,
“Geo”
NLNL/ New London Nucleonics Laboratory
Copyright © Viscom
Inc. 2007
The treatise may
under no circumstances be resold or redistributed in either printed, electronic,
or any other forms,
without prior written permission from the author.
Comments, criticism
and questions will be appreciated and may be directed
to
the author by email
to GEOelectronics@
All PHOTOS © by the author unless noted otherwise
"Our progress as a nation can be no swifter than our
progress in education" -- J. F.
Kennedy
"You do not really understand something
unless you can explain it to your grandmother.
__._,_.___